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Angewandte Chemie International Edition, ISSN 1433-7851, 08/2017, Volume 56, Issue 35, pp. 10506 - 10510
A highly active FeSe2 electrocatalyst for durable overall water splitting was prepared from a molecular 2Fe‐2Se precursor. The as‐synthesized FeSe2 was... 
hydrogen evolution | bioinspired complexes | energy conversion | mixed valence | oxygen evolution | CELLS | TISSUE | INJURY | SENSOR | ISCHEMIA | CHEMISTRY, MULTIDISCIPLINARY | LIVE RAT-BRAIN | OXYGEN | METABOLISM | BIOSENSOR | PH VALUES | Hydrogen | Nickel products | Selenide | Water splitting | Oxygen | Stability | Hydrogen evolution | Catalytic activity | Iron | Electrodes | Splitting | Precursors | Nickel | Catalysis | Chemical synthesis | Current density
Journal Article
Journal of the American Chemical Society, ISSN 0002-7863, 12/2018, Volume 140, Issue 49, pp. 16962 - 16966
The first hypercoordinated disilene with the longest SiSi distance (2.623(1) Å) reported to date, the 5,6-bis­(amidinato silylenyl)­acenaphtene (amidinato =... 
Journal Article
Dalton Transactions, ISSN 1477-9226, 01/2017, Volume 46, Issue 47, pp. 16412 - 16418
Reaction of FeX2(thf)n (X = Cl n = 1.5, Br n = 2) with the chelating 1,1′-bis(silylenyl)-substituted ferrocene ligand SiFcSiA (Fc = ferrocendiyl, Si =... 
Parameters | Nuclear magnetic resonance--NMR | Iron 57 | Ketones | Toluene | Iron | Hydrogenation | Aliphatic compounds | Alcohols | Substitutes | Valence | Mathematical analysis | Benzene | Chelation | Ligands | Oxidation | Catalysis | Coordination compounds | Chemical synthesis | Diamagnetism
Journal Article
Angewandte Chemie-International Edition, ISSN 1433-7851, 12/2015, Volume 54, Issue 50, pp. 15060 - 15063
The reaction of the arylchlorosilylene–NHC adduct ArSi(NHC)Cl [Ar=2,6‐Trip2‐C6H3; NHC=(MeC)2(NMe)2C] 1 with one molar equiv of LiPH2.dme... 
PHOSPHANES | ZWITTERIONIC PHOSPHASILENE | X-RAY-STRUCTURE | COMPLEXES | SILICON-PHOSPHORUS | UNUSUAL REACTIVITY | silicon | DOUBLE-BONDS | heavier olefin analogues | CHEMISTRY | zwitterions | HALF-PARENT PHOSPHASILENE | multiple bonds | phosphorus | SI-P | CHEMISTRY, MULTIDISCIPLINARY | Surface active agents
Journal Article
Nature Chemistry, ISSN 1755-4330, 07/2012, Volume 4, Issue 7, pp. 525 - 526
Journal Article
Chemical Society Reviews, ISSN 0306-0012, 06/2018, Volume 47, Issue 11, pp. 4176 - 4197
The chemistry of group 14 element(II) hydride complexes has rapidly expanded since the first stable example of such a compound was reported in 2000. Since that... 
AMBIENT CONDITIONS | HYDROGEN ABSTRACTION | SILICON(II) HYDRIDE | THIOLATE COMPLEXES | OXIDATIVE ADDITION | MAIN-GROUP ELEMENTS | REDUCTIVE ELIMINATION | CARBON-DIOXIDE | CHEMISTRY, MULTIDISCIPLINARY | ORGANOTIN TRIHYDRIDE | UNACTIVATED ALKENES | Organic chemistry | Electronic structure | Reactivity | Design modifications | Ligands | Hydrides | Catalysis | Chemical synthesis | Substrates
Journal Article
Angewandte Chemie International Edition, ISSN 1433-7851, 03/2019, Volume 58, Issue 12, pp. 3715 - 3728
A significant number of isolable silylenes are currently known. They have quickly developed from laboratory curiosities to useful ligands in metal‐mediated... 
regioselectivity | chemoselectivity | multidentate ligands | stereoselectivity | hydrogenation | DONOR | SILICON | HYDROSILYLATION | BIS(SILYLENE) | N-HETEROCYCLIC SILYLENE | REACTIVITY | CHEMISTRY, MULTIDISCIPLINARY | COMPLEXES SYNTHESIS | 2-COORDINATE | BOND ACTIVATION | BORYLATION | Chemotherapy | Catalysis | Hydrogenation | Cancer | Steering | Amination | Phosphine | Metals | Ligands | Hydrosilylation | Transformations | Deuteration
Journal Article
Angewandte Chemie International Edition, ISSN 1433-7851, 07/2013, Volume 52, Issue 28, pp. 7147 - 7150
King of donor: The chelating bis(carbene) 1 enabled the synthesis of the new silyliumylidene salt 2. This salt can be dechlorinated with sodium naphthalenide... 
silyliumylidenes | silicon | main‐group chemistry | siladicarbenes | silylenes | main-group chemistry | STABLE SILYLENE | CONVERSION | MAIN-GROUP | REACTIVITY | DIVALENT CARBON CHEMISTRY | CHEMISTRY, MULTIDISCIPLINARY | ISOLABLE DIALKYLSILYLENE | LIGAND | Silicon | Dechlorination | Chelating | Synthesis | Sodium | Mathematical analysis | Basicity
Journal Article
Phosphorus, Sulfur, and Silicon and the Related Elements, ISSN 1042-6507, 11/2018, Volume 193, Issue 11, pp. 740 - 743
This is for Bob, and for his vast number of friends and colleagues who wish to celebrate his 90 th birthday. On this occasion we express our admiration,... 
reflection | Tribute | organosilicon
Journal Article
Chemical Communications, ISSN 1359-7345, 2018, Volume 54, Issue 67, pp. 9352 - 9355
The unusual reactivity of the SiN bond in metallo-iminosilane [DippN = Si(OSiMe3)Ni(Cl)(NHC)2]1towards CO2and cyclohexyl isocyanate (CyNCO) is reported; it... 
Isocyanates | Cycloaddition | Carbon dioxide | Polarity | Cleavage | Metallography | Silicon | Nickel | Coordination compounds | Crystallography
Journal Article
Angewandte Chemie International Edition, ISSN 1433-7851, 12/2013, Volume 52, Issue 50, pp. 13206 - 13210
Yes, we CAN: Partial oxidation of inactive MnO nanoparticles by CeIV as oxidant gives active MnOx catalysts that are suitable for effective photochemical and... 
oxygen evolution reaction | electrochemistry | water splitting | photochemistry | metal oxide catalysis | RAY-ABSORPTION SPECTROSCOPY | OXIDIZING CATALYST | COMPLEX | RESOLUTION | MODEL | CHEMISTRY, MULTIDISCIPLINARY | MANGANESE OXIDE | OXYGEN REDUCTION | PHOTOSYSTEM-II | CHEMISTRY | PHOTOSYNTHESIS | Electrochemistry | Electrochemical reactions | Corrosion and anti-corrosives
Journal Article
Organometallics, ISSN 0276-7333, 09/2009, Volume 28, Issue 17, pp. 5032 - 5035
Conversion of the β-diketiminato Ge(II) chloride LGeCl [L = CH{CMe(NAr)}2, Ar = 2,6-iPr2C6H3] (1) and its tin homologue LSnCl (2) with the anionic iron complex... 
Journal Article
Chemistry – A European Journal, ISSN 0947-6539, 01/2010, Volume 16, Issue 4, pp. 1281 - 1288
A series of N‐heterocyclic carbene‐stabilized silanechalcogenones 2 a,b (SiO), 3 a,b (SiS), 4 a,b (SiSe), and 5 a,b (SiTe) are described. The silanone... 
carbenes | silanones | chalcogens | multiple bonds | heterocycles | Heterocycles | Multiple bonds | Chalcogens | Silanones | Carbenes | STABLE SILYLENE | SERIES | SILANETHIONE | SILICON | REACTIVITY | CHEMISTRY, MULTIDISCIPLINARY | CHEMISTRY | CHARACTER | DOUBLE-BOND | Spectrum analysis
Journal Article
Energy & Environmental Science, ISSN 1754-5692, 01/2018, Volume 11, Issue 5, pp. 1287 - 1298
The design and development of economical and highly efficient electrocatalysts for the hydrogen evolution reaction (HER) and oxygen evolution reaction (OER)... 
Water splitting | Structural stability | Electrocatalysts | Inorganic materials | Hydrogen evolution | Phosphorus | Inorganic salts | Durability | Heavy metals | Splitting | Anions | Bimetals | Alkaline water | Electrolysis | Nickel | Cations | Catalysis | Chemical evolution
Journal Article
Angewandte Chemie International Edition, ISSN 1433-7851, 10/2016, Volume 55, Issue 41, pp. 12868 - 12872
Journal Article
Journal of the American Chemical Society, ISSN 0002-7863, 02/2019, Volume 141, Issue 7, pp. 3304 - 3314
The synthesis and tautomerization of a "half-parent" aminosilylene and its heavy P- and As-analogues ( LSi-EH ; E = N, P, As; L = N(SiMe )(2,6- Pr C H )) in... 
Journal Article