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by Yamagami, Keitaro and Kurogi, Ryota and Kurogi, Ai and Nishimura, Hiroyuki and Nishimura, Shinjitsu and Nishimura, Yasuaki and Nishimura, Kunihiro and Nishimura, Ataru and Onozuka, Daisuke and Ren, Nice and Kada, Akiko and Arimura, Koichi and Ido, Keisuke and Mizoguchi, Masahiro and Sakamoto, Seisaburo and Sakamoto, Tetsuya and Kayama, Takamasa and Suzuki, Nozomi and Suzuki, Michiyasu and Suzuki, Sachio and Suzuki, Hidenori and Suzuki, Ichiro and Suzuki, Susumu and Arai, Yoshinori and Arai, Hajime and Arai, Motohiro and Hagihara, Akihito and Iihara, Koji and Takigami, Masayoshi and Kamiyama, Kenji and Houkin, Kiyohiro and Nishi, Shougo and Yoshimoto, Tetsuyuki and Yoshimoto, Junpei and Kaneko, Sadao and Oka, Hirofumi and Oka, Koji and Ooyama, Hiroshi and Kamada, Kyousuke and Makino, Kenichi and Tokumitsu, Naoki and Sako, Kazuhiro and Izumi, Naoto and Nitta, Hisashi and Nitta, Kazumi and Ootaki, Masahumi and Isobe, Masanori and Nishiya, Mikio and Yamazaki, Takaaki and Mabuchi, Syouji and Mabuchi, Eiichiro and Ogasawara, Kuniaki and Kubo, Naohiko and Shimizu, Yukihiko and Saito, Hitoshi and Saito, Keiichi and Yamanome, Tatumi and Yoshino, Kimihiro and Yoshino, Atsuo and Fujitsuka, Mitsuyuki and Takami, Masaaki and Ohtaka, Hirotoshi and Hirano, Teruyuki and Shiokawa, Yosiaki and Okada, Takaharu and Kohno, Michihiro and Haraoka, Jou and Kawamura, Noriyoshi and Kawamura, Tadao and Isoshima, Akira and Yasue, Masaharu and Takayoshi Kobayashi, Mitsuhiko Hokari and Kawai, Kensuke and Maehara, Taketoshi and Noguchi, Makoto and Hoshino, Haruhiko and Hiyama, Hirofumi and Yoshida, Kensaku and Yoshida, Kazunari and Utsugi, Osamu and Takeda, Yasuaki and Takeda, Yuu and Tamaki, Kouichi and Karasudani, Hirohide and Urabe, Takao and Kobayashi, Nozomu and Kobayashi, Shiro and Nakamura, Yusaku and Nakamura, Kazuhito and Nakamura, Michio and Nakamura, Yoshinari and Koguchi, Yorio and Ono, Junichi and Suda, Sumio and Hadeishi, Hiromu and Fukutake, Toshio and Wakui, Kenji and Tanno, Hirokazu and Ishige, Naoki and Ohasi, Takashi and ... and J-ASPECT Study Collaborators
World Neurosurgery, ISSN 1878-8750, 10/2019, Volume 130, pp. e26 - e46
The epidemiology of patients with traumatic brain injury (TBI) has changed dramatically over recent decades as a result of rapid advances in aging societies.... 
Aging | Hospital mortality | Prognosis | Traumatic brain injury | Subdural hematoma | SURGERY | CARE | CLINICAL NEUROLOGY | IMPACT | CLINICAL-VARIABLES | HOSPITAL VOLUME | GENDER | COMA
Journal Article
Chemical Reviews, ISSN 0009-2665, 09/2015, Volume 115, Issue 17, p. 9207
  Convergent strategies in the total synthesis of biologically active terpenoids are detailed. New substrates have been developed by chemists using... 
Organic chemistry | Chemical engineering | Chemical bonds | Chemical synthesis | Carbon
Journal Article
Chemical Reviews, ISSN 0009-2665, 09/2015, Volume 115, Issue 17, pp. 9207 - 9231
Convergent strategies in the total synthesis of biologically active terpenoids are detailed. New substrates have been developed by chemists using biosynthetic... 
Synthesis | Chemists | Strategy
Journal Article
Angewandte Chemie International Edition, ISSN 1433-7851, 11/2015, Volume 54, Issue 48, pp. 14457 - 14461
The complex ABC‐tricyclic structure of crotophorbolone, a derivative of the tigliane diterpenoids, was assembled by coupling of simple fragments. The... 
radical reactions | natural products | terpenoids | total synthesis | cross‐coupling | cross-coupling | ORGANIC-SYNTHESIS | LATENT HIV | PROSTRATIN | PHORBOL | CHEMISTRY, MULTIDISCIPLINARY | DENSITY FUNCTIONALS | RADICAL CHEMISTRY | TUMOR PROMOTERS | TIGLIANE RING-SYSTEM | DIMETHYL(METHYLENE)AMMONIUM IODIDE | CARBOXYLIC-ACIDS
Journal Article
Angewandte Chemie International Edition, ISSN 1433-7851, 01/2020, Volume 59, Issue 1, pp. 479 - 486
Talatisamine (1) is a member of the C19‐diterpenoid alkaloid family, and exhibits K+ channel inhibitory and antiarrhythmic activities. The formidable synthetic... 
terpenoids | total synthesis | cyclization | rearrangement | alkaloids
Journal Article
World Journal of Surgery, ISSN 0364-2313, 1/2018, Volume 42, Issue 1, pp. 185 - 194
Journal Article
2013, ISBN 9780080993621, Volume 9, 27
In this chapter, we described the asymmetric total synthesis of merrilactone A and resolvin E2 based on the symmetry-driven strategy. The enantio- and... 
Asymmetric total synthesis | Pairwise functionalizations | Natural products | Merrilactone A | meso-compound | Desymmetrization | Resolvin E2 | Transannular aldol reaction | Enantioselective solvolysis | Organic compound synthesis
Book Chapter
Journal of Antibiotics, ISSN 0021-8820, 02/2018, Volume 71, Issue 2, pp. 326 - 332
C19-diterpene alkaloids are a class of alkaloids with pharmacologically important activities having an intricately fused hexacyclic ABCDEF-ring system. Here we... 
ALCOHOLS | TALATISAMINE | BIOTECHNOLOGY & APPLIED MICROBIOLOGY | DITERPENOID ALKALOIDS | NATURAL-PRODUCTS | CONSTRUCTION | BRIDGEHEAD RADICALS | CARBONYL-COMPOUNDS | MICROBIOLOGY | PHARMACOLOGY & PHARMACY | IMMUNOLOGY | STRATEGIES
Journal Article
Organic Letters, ISSN 1523-7060, 10/2013, Volume 15, Issue 19, pp. 5122 - 5125
Et3B-mediated three-component coupling reactions between O,Te-acetal, α,β-unsaturated ketones, and aldehydes/ketones were developed. Et3B promoted the... 
Stereoisomerism | Boranes - chemistry | Ketones - chemistry | Molecular Structure | Tellurium - chemistry | Acetals | Aldehydes - chemistry
Journal Article
Tetrahedron Letters, ISSN 0040-4039, 03/2019, Volume 60, Issue 13, p. 885
Iron-catalyzed [delta]-selective conjugate addition of methyl and cyclopropyl Grignard reagents to [alpha],[beta],[gamma],[delta]-unsaturated esters and amides... 
Chemical tests and reagents | Cyclopropane compounds | Amides | Esters | Methylation
Journal Article
ANZ Journal of Surgery, ISSN 1445-1433, 09/2019, Volume 89, Issue 9, pp. 1166 - 1167
Journal Article
Tetrahedron, ISSN 0040-4020, 12/2016, Volume 72, Issue 48, pp. 7839 - 7848
Et B/O -mediated radical coupling reactions of O,Te-acetal were explored using diverse electrophilic double bonds. Ethyl radical derived from Et B under air... 
Organotellurium compounds | Triethylborane | Radical reactions | α-alkoxy bridgehead radical | C–C bond formation
Journal Article
ANZ Journal of Surgery, ISSN 1445-1433, 06/2019, Volume 89, Issue 6, pp. 784 - 785
Journal Article
Bulletin of the Chemical Society of Japan, ISSN 0009-2673, 10/2016, Volume 89, Issue 10, p. 1137
This account describes the development of a synthetic route to crotophorbolone (1). Compound 1 is classified as a derivative of the tigliane diterpenoids, and... 
Stereoselectivity | Saturn | Chemical reactions | Functional groups
Journal Article
Tetrahedron, ISSN 0040-4020, 06/2017, Volume 73, Issue 26, p. 3596
A Cu-catalyzed radical reaction of Cl.sub.2C(CN).sub.2 was utilized for stereoselective conversion of unsaturated molecules into functionalized carbocycles.... 
Chemotherapy | Dioxane | Cancer
Journal Article
Tetrahedron, ISSN 0040-4020, 06/2017, Volume 73, Issue 26, pp. 3596 - 3605
A Cu-catalyzed radical reaction of Cl C(CN) was utilized for stereoselective conversion of unsaturated molecules into functionalized carbocycles.... 
Cascade reaction | Decalin | Stereoselectivity | Carbocycles | Radical reaction
Journal Article
ISSN 1359-7345, 4/2017, Volume 53, Issue 29, pp. 473 - 476
A synthetic route to the septahydroxylated ABC-ring system of dihydro-β-agarofurans was established. The B-ring was formed by a base-promoted... 
Journal Article
The Journal of Organic Chemistry, ISSN 0022-3263, 11/2016, Volume 81, Issue 21, pp. 10204 - 10213
The fused 6/7/5/6/6-membered (ABCDE) ring system of talatisamine was synthesized in 22 steps. After preparation of the AE-ring structure from... 
OXIDATION | ALCOHOLS | ALKENES | ANALOGS | CHEMISTRY, ORGANIC | STEREOSPECIFIC TOTAL-SYNTHESIS | IONS | GENERATION | CHASMANINE | BLOCKER | ALKALOIDS | Usage | Amines | Chemical properties | Ring formation (Chemistry) | Chemical synthesis
Journal Article
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