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Angewandte Chemie, ISSN 0044-8249, 08/2017, Volume 129, Issue 36, pp. 11064 - 11067
The palladium(II)‐catalyzed C(sp3)−H alkynylation of oligopeptides was developed with tetrabutylammonium acetate as a key additive. Through molecular design,... 
Palladium | Peptide | Alkinylierungen | Wirkstoffkonjugation | C-H-Aktivierung
Journal Article
Angewandte Chemie, ISSN 0044-8249, 03/2016, Volume 128, Issue 11, pp. 3818 - 3821
Oxidation of zero‐valent phosphine complexes [M(PtBu3)2] (M=Pd, Pt) has been investigated in 1,2‐difluorobenzene solution using cyclic voltammetry and... 
Phosphanliganden | Palladium | Oxidationen | Platin | C-H-Aktivierung
Journal Article
Angewandte Chemie, ISSN 0044-8249, 01/2018, Volume 130, Issue 5, pp. 1408 - 1412
Previous enantioselective Pd0‐catalyzed C−H activation reactions proceeding via the concerted metalation‐deprotonation mechanism employed either a chiral... 
Arylierungen | Palladium | Asymmetrische Katalyse | P-Liganden | C-H-Aktivierung | Enantiomers
Journal Article
Angewandte Chemie, ISSN 0044-8249, 11/2017, Volume 129, Issue 47, pp. 15327 - 15331
The para‐selective C−H alkylation of aniline derivatives furnished with a pyrimidine auxiliary is herein reported. This reaction is proposed to take place via... 
Arene | Homogene Katalyse | Ruthenium | Reaktionsmechanismen | C-H-Aktivierung | Aniline
Journal Article
Angewandte Chemie, ISSN 0044-8249, 10/2017, Volume 129, Issue 42, pp. 13297 - 13301
The functionalization of carbon–hydrogen bonds in non‐nucleophilic substrates using α‐carbonyl sulfoxonium ylides has not been so far investigated, despite the... 
Schwefel | Homogene Katalyse | Rhodium | C-H-Aktivierung | Ylide
Journal Article
Angewandte Chemie - International Edition, ISSN 0570-0833, 2017, Volume 56, Issue 25, pp. 7161 - 7271
Described herein is an effective and practical modular flow design for the meta‐selective C−H arylation of anilines. The design consists of four... 
Arylierungen | Hypervalente Verbindungen | Kupfer | C-H-Aktivierung | Flusschemie | Aniline | Chromatography
Journal Article
Angewandte Chemie, ISSN 0044-8249, 09/2016, Volume 128, Issue 40, pp. 12643 - 12647
Manganese‐catalyzed C−H bond activation chemistry is emerging as a powerful and complementary method for molecular functionalization. A highly reactive... 
Nachhaltigkeit | Katalyse | Funktionalisierungen | Mangan | C-H-Aktivierung | Pathways | Activation | Substrates
Journal Article
Angewandte Chemie, ISSN 0044-8249, 10/2019, Volume 131, Issue 42, pp. 14966 - 14991
Dieser Aufsatz gibt einen aktuellen Überblick über Fluorierungen per C(sp2)‐H‐ und C(sp3)‐H‐Aktivierung. Übergangsmetallkatalysierte Methoden haben den regio‐... 
Radikalchemie | Übergangsmetallkatalyse | Radiochemie | C-H-Aktivierung | Fluorierung
Journal Article
Angewandte Chemie, ISSN 0044-8249, 01/2019, Volume 131, Issue 1, pp. 308 - 312
Disclosed herein is the merging of C−H activation and radical chemistry, enabling rapid access to a structurally diverse family of fused carbohelicenes through... 
Carbohelicene | Anellierungen | Radikalreaktionen | Rhodium-Katalyse | C-H-Aktivierung | Organic chemistry | Activation | Regioselectivity | Chemical synthesis | Alkynes
Journal Article
Angewandte Chemie, ISSN 0044-8249, 06/2013, Volume 125, Issue 23, pp. 6159 - 6162
Amin trifft Aren: Ein Verfahren zur direkten Aminierung von β‐sp2‐C‐H‐Bindungen in Benzoesäuren und γ‐sp2‐C‐H‐Bindungen in Benzylaminen wurde entwickelt. Die... 
Arene | C‐H‐Aktivierung | Aminierungen | Kupfer
Journal Article
Angewandte Chemie, ISSN 0044-8249, 07/2018, Volume 130, Issue 30, pp. 9569 - 9573
A general synthesis of highly substituted 2‐naphthols based on a new carbanionic reaction sequence is demonstrated. The reaction exploits the dual nature of... 
Naphthole | Lithiierungen | Cyclisierungen | Metallierungen | C-H-Aktivierung | Coumarins | Substitutes | Lithium | Chemical synthesis | Aromatic compounds | Ring opening
Journal Article
Angewandte Chemie, ISSN 0044-8249, 10/2017, Volume 129, Issue 43, pp. 13536 - 13540
Selective functionalization at the meta position of arenes remains a significant challenge. In this work, we demonstrate that a single anionic bipyridine... 
Regioselektivität | Homogene Katalyse | Wasserstoffbrücken | Nichtkovalente Wechselwirkungen | C-H-Aktivierung | Surface active agents | Hydrogen | Amides
Journal Article
Angewandte Chemie, ISSN 0044-8249, 10/2017, Volume 129, Issue 43, pp. 13591 - 13595
Methane represents the major constituent of natural gas. It is primarily used only as a source of energy by means of combustion, but could also serve as an... 
Gold | Schwingungsspektroskopie | Ab-initio-Rechnungen | Clusterverbindungen | C-H-Aktivierung | Methane | Combustion | Catalysis | Natural gas
Journal Article