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Chemical Communications, ISSN 1359-7345, 10/2013, Volume 49, Issue 92, pp. 10817 - 10819
DTBP (di-tert-butyl peroxide) is utilized to mediate oxidative 1,2-difunctionalization of activated alkenes with an aryl C(sp(2))-H bond and a benzylic... 
FUNCTIONALIZATION | AMINATION | ARYLALKYLATION | C-H BOND | CARBON | C(SP3)H BOND | OXINDOLES | AMIDATION | CLEAVAGE | CHEMISTRY, MULTIDISCIPLINARY | Indoles - chemical synthesis | Alkenes - chemistry | Cyclohexanes - chemistry | Molecular Structure | Oxidation-Reduction | Indoles - chemistry | Lewis acid | Synthesis | Alkenes | Aromatic compounds | Chemical bonds | Strategy | Peroxides
Journal Article
Organic Letters, ISSN 1523-7060, 11/2011, Volume 13, Issue 21, pp. 5928 - 5931
A general protocol for direct transformation of unreactive C(sp3)–H bonds to C(sp3)–CN bonds has been developed. The C–H activation was effected by... 
CYANIERUNG | ETHERS | NITRILE | NUCLEOPHILIC-SUBSTITUTION | C-C | CHEMISTRY, ORGANIC | METAL | OXIDATIVE CYANATION | CYANIDE | MOLECULAR-OXYGEN | Molecular Structure | Cyanides - chemistry | Free Radicals - chemistry | Hydrogen - chemistry | Photochemical Processes | Proline - chemistry
Journal Article
Journal of the American Chemical Society, ISSN 0002-7863, 10/2012, Volume 134, Issue 39, pp. 16163 - 16166
The cascade oxidative annulation reactions of benzoylacetonitrile with internal alkynes proceed efficiently in the presence of a rhodium catalyst and a copper... 
FUNCTIONALIZATION | O BOND | COUPLING REACTIONS | REGIOSELECTIVE SYNTHESIS | ARYL KETONES | INTERNAL ALKYNES | C-H ACTIVATION | ISOQUINOLONE SYNTHESIS | CHEMISTRY, MULTIDISCIPLINARY | BENZOIC-ACIDS | CARBON ACIDS
Journal Article
Organic Letters, ISSN 1523-7060, 09/2017, Volume 19, Issue 18, pp. 4782 - 4785
The development of the oxidative cross-coupling of unreactive C­(sp3)–H bonds with (hetero)­arene C­(sp2)–H bonds is considerably appealing, yet conceptually... 
FUNCTIONALIZATION | ACTIVATION | HETEROCYCLES | ASSISTANCE | HETEROARYLATION | AMIDATION | CHEMISTRY, ORGANIC | SCAFFOLDS | C-H BONDS | ACCESS | CATALYZED ARYLATION
Journal Article
Journal of the American Chemical Society, ISSN 0002-7863, 1900, Volume 137, Issue 15, pp. 4924 - 4927
The direct carbonylation of aromatic sp2 and unactivated sp3 C–H bonds of amides was achieved via nickel/copper catalysis under atmospheric O2 with the... 
OXIDATIVE CARBONYLATION | ALIPHATIC AMIDES | FUNCTIONALIZATION | PALLADIUM | ACTIVATION | N,N-DIMETHYLFORMAMIDE | DIRECT ARYLATION | COUPLING REACTIONS | CHEMISTRY, MULTIDISCIPLINARY | C-H BONDS | DEHYDROGENATIVE CYCLIZATION
Journal Article
Organic Letters, ISSN 1523-7060, 10/2018, Volume 20, Issue 20, pp. 6420 - 6424
A nickel-catalyzed cross-dehydrogenative coupling reaction of α-C­(sp3)–H bonds in N-methylamides with C­(sp3)–H bonds from cyclic alkanes has been developed,... 
FUNCTIONALIZATION | ACTIVATION | METHYLATION | C-H BOND | OXIDATIVE IODINATION | AMIDATION | CHEMISTRY, ORGANIC | 2-PYRIDONATE TANTALUM COMPLEXES | ALPHA | INTERMOLECULAR HYDROAMINOALKYLATION | AMIDES
Journal Article
Journal of the American Chemical Society, ISSN 0002-7863, 10/2011, Volume 133, Issue 41, pp. 16410 - 16413
Journal Article
Journal of the American Chemical Society, ISSN 0002-7863, 02/2014, Volume 136, Issue 5, pp. 1789 - 1792
The direct alkylation of unactivated sp3 C–H bonds of aliphatic amides was achieved via nickel catalysis with the assist of a bidentate directing group. The... 
PALLADIUM | CROSS-COUPLING REACTIONS | STEREOSPECIFIC FORMATION | SN BONDS | ACTIVATION | C-H BOND | O BOND | NEUTRAL ENDOPEPTIDASE | OXIDATIVE ADDITION | CHEMISTRY, MULTIDISCIPLINARY | GRIGNARD-REAGENTS | Chemical bonds | Nickel | Research | Analysis | Alkylation
Journal Article
Organic Letters, ISSN 1523-7060, 09/2017, Volume 19, Issue 17, pp. 4676 - 4679
Catalytic oxidative cross-dehydrogenative coupling between unactivated C­(sp2)–H and C­(sp3)–H bonds is achieved by the cobalt-catalyzed o-alkylation reaction... 
DIRECTING GROUPS | CYCLOALKANES | ACTIVATION | C-H BOND | FUNCTIONALIZATIONS | RINGS | ARENES | ARYLATION | ESTERS | CHEMISTRY, ORGANIC | DERIVATIVES
Journal Article
Journal of the American Chemical Society, ISSN 0002-7863, 05/2012, Volume 134, Issue 17, pp. 7313 - 7316
We report the efficient synthesis of alkyl ethers by the functionalization of unactivated sp3- and sp2-hybridized C–H bonds. In the Pd(OAc)2-catalyzed,... 
FUNCTIONALIZATION | OXIDATION | OXYGEN | CROSS-COUPLING REACTIONS | ORGANIC-MOLECULES | CARBON | C-O | H INSERTION | ARYL | FORMING REDUCTIVE ELIMINATION | CHEMISTRY, MULTIDISCIPLINARY
Journal Article
Journal of the American Chemical Society, ISSN 0002-7863, 02/2019, Volume 141, Issue 7, pp. 2800 - 2813
Radical fragment coupling reactions that unite intricate subunits have become an important class of transformations within the arena of complex molecule... 
ORGANIC-SYNTHESIS | COUPLING REACTIONS | INTERMOLECULAR ADDITION | NATURAL-PRODUCTS | ENANTIOSELECTIVE TOTAL SYNTHESES | CONSTRUCTION | LIGHT PHOTOREDOX CATALYSIS | OLEFINS | REDOX-ACTIVE ESTERS | CONCISE SYNTHESIS | CHEMISTRY, MULTIDISCIPLINARY | Total Synthesis | Radical Chemistry | Natural Products | Fragment Coupling | C-C Bond Formation
Journal Article
Chemical Science, ISSN 2041-6520, 2016, Volume 7, Issue 2, pp. 1383 - 1387
An efficient method of selective beta-arylation of oxime ethers was realized by using a palladium catalyst with diaryliodonium salts as the key arylation... 
FUNCTIONALIZATION | COUPLING REACTIONS | PIVALIC ACID | HYDRIDE ELIMINATION | POLYVALENT IODINE | ARYL IODIDES | REDUCTIVE ELIMINATION | CHEMISTRY, MULTIDISCIPLINARY | C-H BONDS | HYDROGEN ELIMINATION | METAL-FREE
Journal Article
Organic Letters, ISSN 1523-7060, 03/2015, Volume 17, Issue 5, pp. 1340 - 1343
The nickel-catalyzed β-thioetherification of unactivated C(sp3)–H bond of propionamides is established with the assistance of 8-aminoquinoline auxiliary,... 
FUNCTIONALIZATION | UNACTIVATED C(SP)-H BONDS | C(SP)-H BONDS | ACTIVATION | DIRECT ARYLATION | OLEFINATION | INTRAMOLECULAR AMINATION | CHEMISTRY, ORGANIC | STEREOSELECTIVE-SYNTHESIS | C-H BONDS | ALKYL-HALIDES
Journal Article
Journal of the American Chemical Society, ISSN 0002-7863, 01/2014, Volume 136, Issue 3, pp. 1062 - 1069
In recent years a significant progress has been made for the carboxylation of aryl and benzyl halides with CO2, becoming convenient alternatives to the use of... 
ORGANOZINC REAGENTS | CROSS-COUPLING REACTIONS | ACTIVATION | COMPLEX | C-O BOND | H BONDS | ARYL | METAL | BUILDING-BLOCK | CARBON-DIOXIDE | CHEMISTRY, MULTIDISCIPLINARY
Journal Article
Chemical science, ISSN 2041-6520, 03/2017, Volume 8, Issue 3, pp. 2431 - 2435
A general efficient regioselective cobalt catalyzed carbonylation of unactivated C(sp )-H bonds of aliphatic amides was demonstrated using atmospheric (1-2... 
Journal Article
Journal of the American Chemical Society, ISSN 0002-7863, 08/2011, Volume 133, Issue 33, pp. 12984 - 12986
The first catalytic alkynylation of unactivated C(sp3)–H bonds has been accomplished. The method allows for the straightforward introduction of an ethynyl... 
FUNCTIONALIZATION | ACTIVATION | GACL3-CATALYZED ORTHO-ETHYNYLATION | COUPLING REACTIONS | ARYLATION | TERMINAL ALKYNES | COPPER | CARBON-HYDROGEN BONDS | DIRECT ALKYNYLATION | CHEMISTRY, MULTIDISCIPLINARY | C-H BONDS | Alkynes - chemistry | Catalysis | Palladium - chemistry | Carboxylic Acids - chemistry
Journal Article
Organic Letters, ISSN 1523-7060, 09/2016, Volume 18, Issue 17, pp. 4388 - 4391
A transition metal (TM)-free practical synthesis of biologically relevant benzoxazinones has been established via a selective oxidative decarbonylative... 
FUNCTIONALIZATION | C-H BOND | RADICAL PROCESS | ATOM ECONOMY | ONE-POT SYNTHESIS | COUPLING REACTIONS | GREEN CHEMISTRY | ARYLATION | CHEMISTRY, ORGANIC | 4H-3,1-BENZOXAZIN-4-ONES | ARYL
Journal Article
Journal of the American Chemical Society, ISSN 0002-7863, 09/2014, Volume 136, Issue 38, pp. 13194 - 13197
Journal Article
Chemical Science, ISSN 2041-6520, 07/2015, Volume 6, Issue 10, pp. 5978 - 5983
The pyridine-enabled cross dehydrogenative coupling of sp(2) C-H bonds of polyfluoroarenes and unactivated sp(3) C-H bonds of amides was achieved via a... 
DIRECTING GROUP | FUNCTIONALIZATION | PALLADIUM | DIRECT ARYLATION | INTRAMOLECULAR AMINATION | BENZOIC-ACID DERIVATIVES | ELECTRON-DEFICIENT ARENES | CATALYZED DIRECT THIOLATION | CHEMISTRY, MULTIDISCIPLINARY | C-H BONDS | GENERAL-METHOD
Journal Article
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