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Angewandte Chemie International Edition, ISSN 1433-7851, 04/2018, Volume 57, Issue 17, pp. 4804 - 4804
The combination of an allenyne with an additional π‐component in the presence of a rhodium(I) catalyst constitutes a new approach for ring closure. In their... 
allenes | C−C activation | cycloisomerization | alkynes | rhodium
Journal Article
Angewandte Chemie - International Edition, ISSN 1433-7851, 08/2015, Volume 54, Issue 35, pp. 10280 - 10283
Journal Article
Angewandte Chemie International Edition, ISSN 1433-7851, 12/2012, Volume 51, Issue 50, pp. 12559 - 12563
A two‐metal job: Four‐coordinate aluminum dihydrides such as 1 are reported as terminal reductants for the selective title reaction. The heterobimetallic... 
hydrides | aluminum | zirconocene | CF activation | synthetic methods | C-F activation
Journal Article
Journal of the American Chemical Society, ISSN 0002-7863, 02/2019, Volume 141, Issue 7, pp. 2800 - 2813
Radical fragment coupling reactions that unite intricate subunits have become an important class of transformations within the arena of complex molecule... 
ORGANIC-SYNTHESIS | COUPLING REACTIONS | INTERMOLECULAR ADDITION | NATURAL-PRODUCTS | ENANTIOSELECTIVE TOTAL SYNTHESES | CONSTRUCTION | LIGHT PHOTOREDOX CATALYSIS | OLEFINS | REDOX-ACTIVE ESTERS | CONCISE SYNTHESIS | CHEMISTRY, MULTIDISCIPLINARY | Total Synthesis | Radical Chemistry | Natural Products | Fragment Coupling | C-C Bond Formation
Journal Article
Chemistry (Weinheim an der Bergstrasse, Germany), 11/2018, Volume 24, Issue 61, p. 16282
sp C-F Bonds of fluoroalkanes (7 examples; 1°, 2° and 3°) undergo addition to a low-valent Mg-Mg species generating reactive organomagnesium reagents. Further... 
Journal Article
Journal of the American Chemical Society, ISSN 0002-7863, 09/2016, Volume 138, Issue 37, pp. 12061 - 12064
A novel strategy for the synthesis of functionalized carbocycles is defined, through the cascade carbocylization of alkenylboronic acids with delta- or... 
TERTIARY BORONIC ESTERS | INSERTION | CARBON | CATALYZED SYNTHESIS | ALLYLBORATION | C-C BOND | CASCADE | ALDEHYDES | STEREOGENIC CENTERS | CHEMISTRY, MULTIDISCIPLINARY | HYDROACYLATION
Journal Article
Angewandte Chemie, ISSN 0044-8249, 04/2018, Volume 130, Issue 17, pp. 4896 - 4896
Die Kombination eines Allenins …… mit einer zusätzlichen π‐Komponente in Gegenwart eines Rhodium(I)‐Katalysators ermöglicht einen neuartigen Ringschluss. In... 
C-C-Aktivierung | Allene | Rhodium | Cycloisomerisierungen | Alkine
Journal Article
Organometallics, ISSN 0276-7333, 12/2018, Volume 37, Issue 24, pp. 4699 - 4710
While alkyne insertion into metal-carbon(sp(2)) bonds is common in transition metal chemistry, direct alkyne insertions into E-C(sp(2)) bonds are very rare in... 
ELECTROPHILIC AROMATIC-SUBSTITUTION | PHOSPHIRENE | C-C | CHEMISTRY, ORGANIC | CARBON SIGMA-BONDS | TUNGSTEN(II)-CATALYZED REARRANGEMENTS | OXIDES | MAIN-GROUP ELEMENTS | DERIVATIVES | ELECTROLUMINESCENCE | ALKENYLATION | CHEMISTRY, INORGANIC & NUCLEAR
Journal Article
Organic Letters, ISSN 1523-7060, 06/2012, Volume 14, Issue 12, pp. 3218 - 3221
An unexpected Cu-catalyzed oxidative cleavage of the C(sp(3))-C(sp(3)) bond in glycol ethers by using air or molecular oxygen as the terminal stoichiometric... 
ALCOHOLS | KETONES | ACTIVATION | ACID | C-C BOND | COMPLEXES | ESTERS | REACTIVITY | CHEMISTRY, ORGANIC | CARBON-CARBON BONDS | MOLECULAR-OXYGEN
Journal Article
Angewandte Chemie, ISSN 0044-8249, 04/2018, Volume 130, Issue 17, pp. 4797 - 4801
Upon exposure to a catalytic amount of [RhCl(CO)2]2 in 1,4‐dioxane, homopropargylallene‐alkynes underwent a novel cycloisomerization accompanied by the... 
C-C-Aktivierung | Allene | Rhodium | Cycloisomerisierungen | Alkine | Migration | Isomerization | Catalysis | Functional groups | Substrates | Alkynes
Journal Article
Journal of the American Chemical Society, ISSN 0002-7863, 01/2014, Volume 136, Issue 3, pp. 1062 - 1069
In recent years a significant progress has been made for the carboxylation of aryl and benzyl halides with CO2, becoming convenient alternatives to the use of... 
ORGANOZINC REAGENTS | CROSS-COUPLING REACTIONS | MILD CONDITIONS | AROMATIC HALIDES | C-O BOND | ALKENYLBORONIC ESTERS | BUILDING-BLOCK | CARBON-DIOXIDE | CHEMISTRY, MULTIDISCIPLINARY | GRIGNARD-REAGENTS | PHENOL DERIVATIVES
Journal Article
Journal of the American Chemical Society, ISSN 0002-7863, 03/2018, Volume 140, Issue 11, pp. 3981 - 3987
An efficient protocol was developed to construct functionally dense quaternary carbons with concomitant formation of a new Csp(3)-Csp(3) bond via Pd-catalyzed... 
METAL-FREE SYNTHESIS | CYCLOADDITION | VINYLETHYLENE CARBONATES | C-C | ALPHA-ALLYLATION | ALDEHYDES | ENANTIOSELECTIVE CONSTRUCTION | ALLYLIC SUBSTITUTION | CHEMISTRY, MULTIDISCIPLINARY | TETRASUBSTITUTED OLEFINS | HIGHLY EFFICIENT
Journal Article
Chemical Science, ISSN 2041-6520, 2017, Volume 8, Issue 4, pp. 3002 - 3006
An efficient and convenient synthesis of highly functionalized dihydropyrans has been achieved through rhodium(I)-catalysed tandem C(sp(3))-C(sp(3)) bond... 
TERT-CYCLOBUTANOLS | QUATERNARY STEREOGENIC CENTERS | PRACTICAL SYNTHESIS | ENANTIOSELECTIVE SYNTHESIS | CYCLIZATION REACTIONS | SUBSTITUTED OXETANES | C-C BOND | CARBON-CARBON BONDS | ASYMMETRIC HYDROGENATION | CHEMISTRY, MULTIDISCIPLINARY | MARINE SPONGE | Organic chemistry | Cycloaddition | Synthesis | Chemical bonds | Chemical reactions | Ligands | Cleavage | Alkynes
Journal Article
by Chen, YC and Zhu, MK and Loh, TP
ORGANIC LETTERS, ISSN 1523-7060, 06/2015, Volume 17, Issue 11, pp. 2712 - 2715
A C-C bond cleavage was observed in the palladium-catalyzed aminohydroxylation of allylic hydrazones, using atmospheric oxygen as the sole oxidant. This... 
INTERMOLECULAR AMINOACETOXYLATION | ALKENES | DECARBONYLATION | DIASTEREOSELECTIVE SYNTHESIS | CARBON-CARBON BOND | HOMOALLYL ALCOHOLS | ARYLATION | C-C BONDS | DIAMINATION | CHEMISTRY, ORGANIC | CARBOXYLIC-ACIDS
Journal Article
Angewandte Chemie, ISSN 0044-8249, 07/2019, Volume 131, Issue 31, pp. 10803 - 10807
The selective cleavage of thermodynamically stable C(sp3)−C(sp3) single bonds is rare compared to their ubiquitous formation. Herein, we describe a general... 
Morpholine | Amine | Luft | C-C-Spaltung | Kupfer | Transformation | Amines | Catalysts | Natural products | Amides | Cleavage | Transformations | Catalysis | Functional groups
Journal Article
Chemical Communications, ISSN 1359-7345, 2017, Volume 53, Issue 58, pp. 8196 - 8198
DFT computations reveal different reactionmechanisms for the oxidative addition of C(sp(2))-F and C(sp(3))-F bonds to the Al(I) complexes: a concerted... 
DENSITY | HYDROGEN | AR=2,6-IPRCH | CHEMISTRY | FLUORINE | OLEFINS | SIGMA-BONDS | AL(I) | C-F | CHEMISTRY, MULTIDISCIPLINARY | MOLECULES
Journal Article
INDIAN JOURNAL OF CHEMISTRY SECTION B-ORGANIC CHEMISTRY INCLUDING MEDICINAL CHEMISTRY, ISSN 0376-4699, 04/2018, Volume 57, Issue 4, pp. 523 - 533
A catalyst free protocol for nucleophilic C(sp)2-C(sp)3 bond cleavage of alpha-nitroketone has been achieved for the formation of C-O and C-N bond. A series of... 
AEROBIC OXIDATIVE CLEAVAGE | SELECTIVE OXIDATION | ACTIVATION | CARBON | esters | alpha-nitroketone | C-C BONDS | ESTERIFICATION | CHEMISTRY, ORGANIC | bromamine-T | ALDEHYDES | ALCOHOLS | amide | C-C Cleavage | MOLECULAR-OXYGEN
Journal Article
Journal of the American Chemical Society, ISSN 0002-7863, 12/2017, Volume 139, Issue 51, pp. 18444 - 18447
The conversion of easily available trifluoromethylarenes into aryldifluoromethyl compounds, which are valuable motifs in the pharmaceutical chemistry, is... 
MEDICINAL CHEMISTRY | FUNCTIONALIZATION | FACILE ACCESS | ALKYLATION | ALPHA,ALPHA,ALPHA-TRIFLUOROTOLUENE | FLUORINE | C-F BOND | DERIVATIVES | CHEMISTRY, MULTIDISCIPLINARY | ELECTRON-TRANSFER REACTIONS | HYDRODEFLUORINATION
Journal Article
Journal of Organic Chemistry, ISSN 0022-3263, 05/2019, Volume 84, Issue 10, pp. 6366 - 6376
The first general palladium-catalyzed amination of aryl phosphates is described. The combination of MorDalPhos with [Pd(pi-cinnamyl)Cl](2) enables the... 
ROOM-TEMPERATURE | MONOARYLATION | C-N | AMINES | ARYLATION | CHEMISTRY, ORGANIC | BUCHWALD-HARTWIG AMINATION | AROMATIC AMINATION | EFFICIENT | ARYL CHLORIDES | REDUCTIVE AMINATION
Journal Article
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