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Angewandte Chemie International Edition, ISSN 1433-7851, 05/2010, Volume 49, Issue 23, pp. 3947 - 3951
CF bond borylation: A 16‐electron rhodium(I)–boryl complex was synthesized by borylation of a rhodium(I)–fluorine complex. The former reacts with benzene or... 
CH activation | CF activation | boryl ligands | borylation | rhodium | Boryl ligands | C-H activation | Rhodium | C-F activation | Borylation | TRANSITION-METAL-COMPLEXES | P-C | DEHYDROGENATIVE BORYLATION | OXIDATIVE ADDITION | CHEMISTRY, MULTIDISCIPLINARY | FUNCTIONALIZATION | CARBON-FLUORINE BONDS | COUPLING REACTIONS | DIBORON REAGENTS | B-H | N-HETEROCYCLES
Journal Article
Angewandte Chemie International Edition, ISSN 1433-7851, 04/2012, Volume 51, Issue 14, pp. 3414 - 3417
PdIV–fluoride complexes, some of which are remarkably insensitive to water, have been synthesized and used in the title reaction, which proceeds with high... 
chemoselectivity | palladium | fluorinated ligands | homogeneous catalysis | redox chemistry | CATALYSIS | ACTIVATION | EXPONENT BASIS-SETS | CONVERSION | FLUORINATION | ARYL FLUORIDES | CHEMISTRY, MULTIDISCIPLINARY | CHEMISTRY | C-F BOND | COMPACT EFFECTIVE POTENTIALS | TRIFLUOROMETHYLATION | Pyridines | Joining | Selectivity | Palladium | Pathways | Bonding
Journal Article
Angewandte Chemie International Edition, ISSN 1433-7851, 06/2017, Volume 56, Issue 25, pp. 7266 - 7270
Journal Article
Chemistry – A European Journal, ISSN 0947-6539, 08/2016, Volume 22, Issue 32, pp. 11461 - 11468
Journal Article
Angewandte Chemie International Edition, ISSN 1433-7851, 02/2019, Volume 58, Issue 9, pp. 2804 - 2808
The reaction of SIPr, [1,3‐bis(2,6‐diisopropylphenyl)‐imidazolin‐2‐ylidene] (1), with C6F6 led to the formation of an unprecedented mesoionic compound (2). The... 
ylides | structure elucidation | C−F activation | carbanions | N-heterocyclic carbenes | Lewis acid | Fluoride | Fluorides
Journal Article
Angewandte Chemie International Edition, ISSN 1433-7851, 02/2019, Volume 58, Issue 7, pp. 2064 - 2068
The ability to selectively forge C–heteroatom bonds by C−F scission is typically accomplished by metal catalysts, specialized ligands and/or harsh reaction... 
cross-coupling | reaction mechanisms | silylation | synthetic methods | fluorine | CROSS-COUPLING REACTION | ALPHA-ARYLATION | PALLADIUM-CATALYZED SILYLATION | C-F ACTIVATION | ARYL FLUORIDES | CLEAVAGE | CHEMISTRY, MULTIDISCIPLINARY | NUCLEOPHILIC AROMATIC-SUBSTITUTION | POLYFLUOROARENES | GRIGNARD-REAGENTS | BORYLATION | Metal catalysts | Fluorides | Cleavage | Catalysis | Catalysts | Bonding | Metals
Journal Article
ACS Catalysis, ISSN 2155-5435, 10/2017, Volume 7, Issue 10, pp. 6999 - 7002
Silylium ions facilitate the catalytic direct cross-coupling of aryl fluorides with simple arenes and alkanes. This C–H arylation approach is initiated by... 
C-H bond activation | Main-group catalysis | C-F bond activation | Carbocations | Silylium ions | Cross-coupling | ETHANE | silylium ions | carbocations | CHEMISTRY, PHYSICAL | F ACTIVATION | HYDRODEFLUORINATION | CATIONS | main-group catalysis | METHANE | cross-coupling | BORYLATION
Journal Article
Angewandte Chemie International Edition, ISSN 1433-7851, 05/2017, Volume 56, Issue 21, pp. 5890 - 5893
Activation of the sp3 C−F bond in 2‐trifluoromethyl‐1‐alkenes was accomplished through treatment with a Lewis acid. In the presence of an equimolar amount of... 
Lewis acids | C−F bond activation | allylation | carbocations | fluorine | Olefins | Bonds | Fluorides | Lewis acid | Activation | Fluoride | Alkenes | Acids | Aromatic compounds
Journal Article
Angewandte Chemie International Edition, ISSN 1433-7851, 07/2014, Volume 53, Issue 29, pp. 7564 - 7568
The nickel‐mediated [3+2] cycloaddition of 2‐trifluoromethyl‐1‐alkenes with alkynes afforded fluorine‐containing multi‐substituted cyclopentadienes in a... 
fluoroalkenes | nickel | CF bond activation | cyclopentadienes | cycloaddition | alkynes | VINYLIC FLUORINES | COMPLEXES | EFFICIENT SYNTHESIS | C-F bond activation | ARYL FLUORIDES | SELECTIVE ACTIVATION | CHEMISTRY, MULTIDISCIPLINARY | HYDRODEFLUORINATION | CATALYZED REDUCTIVE COUPLINGS | KUMADA-TAMAO-CORRIU | CYCLIZATIONS | GRIGNARD-REAGENTS
Journal Article
Journal of the American Chemical Society, ISSN 0002-7863, 12/2017, Volume 139, Issue 51, pp. 18444 - 18447
The conversion of easily available trifluoromethylarenes into aryldifluoromethyl compounds, which are valuable motifs in the pharmaceutical chemistry, is... 
MEDICINAL CHEMISTRY | FUNCTIONALIZATION | FACILE ACCESS | ALKYLATION | ALPHA,ALPHA,ALPHA-TRIFLUOROTOLUENE | FLUORINE | C-F BOND | DERIVATIVES | CHEMISTRY, MULTIDISCIPLINARY | ELECTRON-TRANSFER REACTIONS | HYDRODEFLUORINATION
Journal Article