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Angewandte Chemie, ISSN 0044-8249, 08/2017, Volume 129, Issue 36, pp. 11064 - 11067
The palladium(II)‐catalyzed C(sp3)−H alkynylation of oligopeptides was developed with tetrabutylammonium acetate as a key additive. Through molecular design,... 
Palladium | Peptide | Alkinylierungen | Wirkstoffkonjugation | C-H-Aktivierung
Journal Article
Angewandte Chemie, ISSN 0044-8249, 03/2016, Volume 128, Issue 11, pp. 3818 - 3821
Oxidation of zero‐valent phosphine complexes [M(PtBu3)2] (M=Pd, Pt) has been investigated in 1,2‐difluorobenzene solution using cyclic voltammetry and... 
Phosphanliganden | Palladium | Oxidationen | Platin | C-H-Aktivierung
Journal Article
Angewandte Chemie, ISSN 0044-8249, 08/2018, Volume 130, Issue 32, pp. 10320 - 10324
peri‐Disubstituted naphthalenes exhibit interesting physical properties and unique chemical reactivity, due to the parallel arrangement of the bonds to the two... 
Borylierung | Katalyse | Polyaromatische Kohlenwasserstoffe | Naphthalin | C-H-Aktivierung
Journal Article
Angewandte Chemie, ISSN 0044-8249, 01/2018, Volume 130, Issue 5, pp. 1408 - 1412
Previous enantioselective Pd0‐catalyzed C−H activation reactions proceeding via the concerted metalation‐deprotonation mechanism employed either a chiral... 
Arylierungen | Palladium | Asymmetrische Katalyse | P-Liganden | C-H-Aktivierung | Enantiomers
Journal Article
Angewandte Chemie, ISSN 0044-8249, 11/2017, Volume 129, Issue 47, pp. 15327 - 15331
The para‐selective C−H alkylation of aniline derivatives furnished with a pyrimidine auxiliary is herein reported. This reaction is proposed to take place via... 
Arene | Homogene Katalyse | Ruthenium | Reaktionsmechanismen | C-H-Aktivierung | Aniline
Journal Article
Angewandte Chemie, ISSN 0044-8249, 10/2017, Volume 129, Issue 42, pp. 13297 - 13301
The functionalization of carbon–hydrogen bonds in non‐nucleophilic substrates using α‐carbonyl sulfoxonium ylides has not been so far investigated, despite the... 
Schwefel | Homogene Katalyse | Rhodium | C-H-Aktivierung | Ylide
Journal Article
Angewandte Chemie, ISSN 0044-8249, 01/2019, Volume 131, Issue 1, pp. 308 - 312
Disclosed herein is the merging of C−H activation and radical chemistry, enabling rapid access to a structurally diverse family of fused carbohelicenes through... 
Carbohelicene | Anellierungen | Radikalreaktionen | Rhodium-Katalyse | C-H-Aktivierung | Organic chemistry | Activation | Regioselectivity | Chemical synthesis | Alkynes
Journal Article
Angewandte Chemie, ISSN 0044-8249, 07/2018, Volume 130, Issue 30, pp. 9569 - 9573
A general synthesis of highly substituted 2‐naphthols based on a new carbanionic reaction sequence is demonstrated. The reaction exploits the dual nature of... 
Naphthole | Lithiierungen | Cyclisierungen | Metallierungen | C-H-Aktivierung | Coumarins | Substitutes | Lithium | Chemical synthesis | Aromatic compounds | Ring opening
Journal Article
Angewandte Chemie. International Edition, ISSN 1433-7851, 2017, Volume 56, Issue 43, pp. 13406 - 13410
Methane represents the major constituent of natural gas. It is primarily used only as a source of energy by means of combustion, but could also serve as an... 
Gold | Schwingungsspektroskopie | Ab-initio-Rechnungen | Clusterverbindungen | C-H-Aktivierung | Methane | Combustion | Catalysis | Natural gas
Journal Article
Angewandte Chemie, ISSN 0044-8249, 10/2017, Volume 129, Issue 43, pp. 13536 - 13540
Selective functionalization at the meta position of arenes remains a significant challenge. In this work, we demonstrate that a single anionic bipyridine... 
Regioselektivität | Homogene Katalyse | Wasserstoffbrücken | Nichtkovalente Wechselwirkungen | C-H-Aktivierung | Surface active agents | Hydrogen | Amides
Journal Article
Angewandte Chemie, ISSN 0044-8249, 08/2017, Volume 129, Issue 35, pp. 10666 - 10670
The development of new and practical 3‐pentoxythiocarbonyl auxiliaries for IrI‐catalyzed C−H alkylation of azacycles is described. This method allows for the... 
Pentoxythiocarbonyl | Homogene Katalyse | Alkylierungen | N-Heterocyclen | C-H-Aktivierung | Carbamates | Proline
Journal Article
Angewandte Chemie, ISSN 0044-8249, 01/2019, Volume 131, Issue 1, pp. 313 - 317
Herein, we report the first enantioselective annulation of α‐arylidene pyrazolones through a formal C(sp3)−H activation under mild conditions enabled by highly... 
Hedgehog-Inhibitoren | Spiropyrazolone | Asymmetrische Katalyse | Rhodium | C-H-Aktivierung | Organic chemistry | Catalysts | Natural products | Chemical reactions | Activation | Enantiomers | Pyrazolones | Substrates
Journal Article
Angewandte Chemie, ISSN 0044-8249, 06/2017, Volume 129, Issue 25, pp. 7262 - 7266
A highly atom economical and stereoselective synthesis of tetrasubstituted α,β‐unsaturated amides was achieved by a Cp*CoIII‐catalyzed C−H... 
Erste Übergangsmetalllreihe | Homogene Katalyse | Cobalt | Indole | C-H-Aktivierung | Olefins | Acylation
Journal Article
Angewandte Chemie, ISSN 0044-8249, 05/2017, Volume 129, Issue 19, pp. 5347 - 5350
Both aryl components of diaryliodonium salts can be used in a domino one‐pot reaction via in situ generation of a directing group. A number of heterocycles... 
Arylierungen | Iodoniumverbindungen | Stickstoffheterocyclen | C-H-Aktivierung | Aromatic compounds | Cascade chemical reactions
Journal Article