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n-heteroarenes (44) 44
chemistry, multidisciplinary (21) 21
chemistry, organic (20) 20
catalysis (19) 19
heterocycles (14) 14
photoredox catalysis (12) 12
c-h alkylation (10) 10
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pyridines (10) 10
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alkylation (5) 5
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pyridin (5) 5
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nucleophilic dearomatization (4) 4
quinoline (4) 4
single-electron transmetalation (4) 4
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arenes (3) 3
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heteroarenes (3) 3
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minisci reaction (3) 3
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[chim.orga]chemical sciences/organic chemistry (2) 2
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Organic Letters, ISSN 1523-7060, 06/2018, Volume 20, Issue 11, pp. 3229 - 3232
A metal-free photoredox C–H alkylation of heteroaromatics from readily available carboxylic acids using an organic photocatalyst and hypervalent iodine... 
ORGANIC-SYNTHESIS | HETEROCYCLES | CHEMISTRY, ORGANIC | GENERATION | DERIVATIVES | LATE-STAGE FUNCTIONALIZATION | ARYLBORONIC ACIDS | N-(ACYLOXY)PHTHALIMIDES | PHOTOREDOX CATALYSIS | N-HETEROARENES | TRIFLUOROMETHYLATION
Journal Article
ACS Catalysis, ISSN 2155-5435, 06/2017, Volume 7, Issue 6, pp. 4057 - 4061
The direct visible light-mediated C–H alkylation of heteroarenes using aliphatic carboxylic acids is reported. This mild method proceeds at low catalyst... 
Minisci reaction | alkylation | photoredox catalysis | decarboxylation | C-H functionalization | heterocycles | MERGING PHOTOREDOX | CONVERSION | ARYLATION | CHEMISTRY, PHYSICAL | ALPHA-AMINO-ACIDS | ALKYNYLATION | N-HETEROARENES | SO4 | CARBOXYLIC-ACIDS
Journal Article
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, ISSN 1433-7851, 07/2018, Volume 57, Issue 29, pp. 9131 - 9135
Catalysis with earth-abundant transition metals is an option to help save our rare noble-metal resources and is especially interesting when novel reactivity or... 
METHANOL | ALPHA-OLEFINATION | NOBEL LECTURE | SUSTAINABLE SYNTHESIS | TRANSFER HYDROGENATION | alcohols | N-heteroarenes | manganese | CHEMISTRY, MULTIDISCIPLINARY | KETONES | COUPLING REACTIONS | AMINES | PNP PINCER COMPLEXES | dehydrogenation | EFFICIENT | olefination | Dehydrogenation | Cobalt | Alcohols
Journal Article
Organic Letters, ISSN 1523-7060, 2019, Volume 21, Issue 11, pp. 4259 - 4265
A mild, practical protocol for the decarboxylative alkylation of heteroarenes has been accomplished via iron photocatalysis. A diverse range of carboxylic... 
C-H ALKYLATION | VISIBLE-LIGHT | METHYLATION | PHOTOREDOX | ACIDS | CHEMISTRY, ORGANIC | PHOTOCHEMISTRY | PYRIDINE RING | N-HETEROARENES
Journal Article
ACS Catalysis, ISSN 2155-5435, 01/2017, Volume 7, Issue 1, pp. 907 - 911
Journal Article
Angewandte Chemie International Edition, ISSN 1433-7851, 03/2015, Volume 54, Issue 13, pp. 4055 - 4059
Journal Article
Organic Letters, ISSN 1523-7060, 2019, Volume 21, Issue 7, pp. 2441 - 2444
Considering the ubiquitous C(sp(3))-H and the important value of alkylated heteroarenes, developing a universal method for C(sp(3))-H arylation with... 
FUNCTIONALIZATION | C-H ALKYLATION | ETHERS | HETEROCYCLES | COUPLING REACTIONS | CHEMISTRY, ORGANIC | DIRECT C2-ALKYLATION | BOND ACTIVATION | FLUORINATION | DIRECT ALPHA-ARYLATION | N-HETEROARENES
Journal Article
Chemical Science, ISSN 2041-6520, 2017, Volume 8, Issue 11, pp. 7412 - 7418
The functionalization of heteroarenes has been integral to the structural diversification of medicinally active molecules such as quinolines, pyridines, and... 
ALCOHOLS | FUNCTIONALIZATION | C-H ALKYLATION | NUCLEOPHILIC CHARACTER | METHYLATION | QUINOLINE | ELECTRON-TRANSFER | HETEROCYCLES | RADICALS | CHEMISTRY, MULTIDISCIPLINARY | N-HETEROARENES
Journal Article
by Zhao, H and Jin, J
ORGANIC LETTERS, ISSN 1523-7060, 08/2019, Volume 21, Issue 16, pp. 6179 - 6184
A mild, practical method for direct arylation of unactivated C(sp(3))-H bonds with heteroarenes has been achieved via photochemistry. Selectfluor is used as a... 
METHYLATION | ETHERS | BOND FUNCTIONALIZATION | HETEROARYLATION | CHEMISTRY, ORGANIC | LATE-STAGE FUNCTIONALIZATION | CHALLENGES | N-HETEROARENES | DIRECT ALKYLATION | CARBOXYLIC-ACIDS
Journal Article
Journal Article
The Journal of Organic Chemistry, ISSN 0022-3263, 03/2018, Volume 83, Issue 5, pp. 3000 - 3012
An improved, one-pot Minisci reaction has been developed using visible light, an organic photocatalyst, and carboxylic acids as radical precursors via the... 
CATALYSIS | ALKYL RADICALS | HETEROCYCLES | SUBSTITUTIONS | PHOTOCATALYSIS | CHEMISTRY, ORGANIC | QUATERNARY CARBONS | C-H FUNCTIONALIZATION | ELECTRON-TRANSFER MECHANISM | HETEROAROMATIC BASES | N-HETEROARENES | Usage | Catalysts | Scaffolding | Light | Analysis | Chemical reactions | Organic compounds
Journal Article
by Zhao, H and Li, ZL and Jin, J
NEW JOURNAL OF CHEMISTRY, ISSN 1144-0546, 08/2019, Volume 43, Issue 32, pp. 12533 - 12537
A visible light-mediated green protocol for metal-free oxidative coupling of heteroarenes and aliphatic C-H components has been achieved via a radical pathway.... 
C-H ALKYLATION | DEPROTONATION | METHYLATION | HETEROCYCLES | ACIDS | BOND FUNCTIONALIZATION | OXIDATIONS | DECARBOXYLATIVE ALKYLATION | CHEMISTRY, MULTIDISCIPLINARY | LATE-STAGE FUNCTIONALIZATION | N-HETEROARENES
Journal Article
Angewandte Chemie International Edition, ISSN 1433-7851, 07/2018, Volume 57, Issue 29, pp. 9131 - 9135
Catalysis with earth‐abundant transition metals is an option to help save our rare noble‐metal resources and is especially interesting when novel reactivity or... 
alcohols | dehydrogenation | N-heteroarenes | manganese | olefination | Bromine | Hydrogen storage | Transition metals | Alkenes | Alcohol | Iron | Cobalt compounds | Cobalt | Alkylation | Aliphatic compounds | Heavy metals | Alcohols | Substitutes | Aliphatic alcohols | Dehydrogenation | Catalysis | Coordination compounds | Functional groups | Iodine | Manganese
Journal Article
by Huang, CY and Li, JB and Liu, WB and Li, CJ
CHEMICAL SCIENCE, ISSN 2041-6520, 05/2019, Volume 10, Issue 19, pp. 5018 - 5024
Minisci alkylation is of prime importance for its applicability in functionalizing diverse heteroarenes, which are core structures in many bioactive compounds.... 
RADICAL CHEMISTRY | C(SP)-H BONDS | HYDROGEN ABSTRACTION | ALKYL RADICALS | BIMOLECULAR HOMOLYTIC SUBSTITUTION | SIMPLE ALKANES | ENERGY-TRANSFER | C-H FUNCTIONALIZATION | CHEMISTRY, MULTIDISCIPLINARY | DIRECT ALPHA-ARYLATION | N-HETEROARENES
Journal Article
by Tian, WF and Hu, CH and He, KH and He, XY and Li, Y
ORGANIC LETTERS, ISSN 1523-7060, 09/2019, Volume 21, Issue 17, pp. 6930 - 6935
Herein, we have developed visible-light photo-redox-catalyzed decarboxylating carboxylic acids for alkylation of heteroarenes under mild conditions. The... 
FUNCTIONALIZATION | C-H ALKYLATION | MERGING PHOTOREDOX | COUPLING REACTIONS | AMINO-ACIDS | ARYLATION | CHEMISTRY, ORGANIC | HOMOGENEOUS SYSTEM | ALPHA-KETO ACIDS | HETEROAROMATIC BASES | N-HETEROARENES
Journal Article
ORGANIC LETTERS, ISSN 1523-7060, 05/2018, Volume 20, Issue 10, pp. 2853 - 2856
The abilities of dipyrrolyldiketone boron complexes as hydrogen-bonding donor organocatalysts were examined by the Mannich-type reaction of N-acyl... 
ASYMMETRIC CATALYSIS | BF2 COMPLEXES | SUBSTITUTED DIPYRROLYLDIKETONES | ION-PAIRING ASSEMBLIES | ORGANOCATALYSIS | CHEMISTRY, ORGANIC | PLANAR | CONJUGATED MOLECULES | BINDING CATALYSIS | NUCLEOPHILIC DEAROMATIZATION | N-HETEROARENES
Journal Article
SYNTHESIS-STUTTGART, ISSN 0039-7881, 03/2019, Volume 51, Issue 5, pp. 1063 - 1072
The Minisci reaction, which encompasses the radical C-H alkylation of heteroarenes, has undergone revolutionary development in recent years. The application of... 
METHYLATION | ACIDS | ARYLATION | CHEMISTRY, ORGANIC | visible light | C-H FUNCTIONALIZATION | N-HETEROARENES | heteroarenes | radical alkylation | late-stage functionalization | Minisci reaction | photoredox catalysis | ELECTRON-RICH HETEROCYCLES | DECARBOXYLATIVE ALKYLATION | TRIFLUOROMETHYLATION
Journal Article
ACS Catalysis, ISSN 2155-5435, 04/2019, Volume 9, Issue 4, pp. 3413 - 3418
Despite many recent advances in the radical alkylation of electron-deficient heteroarenes since the seminal reports by Minisci and co-workers, methods for the... 
Minisci reaction | heterocycle synthesis | photoredox catalysis | C-H functionalization | radical chemistry | C-H ALKYLATION | CHEMISTRY, PHYSICAL | N-HETEROARENES | FUNCTIONALIZATION | HETEROCYCLES | SUBSTITUTIONS | KINETICS | LIGHT PHOTOREDOX CATALYSIS | CARBOXYLIC-ACIDS
Journal Article
Chemical Communications, ISSN 1359-7345, 2018, Volume 54, Issue 62, pp. 8622 - 8625
A reduction of quinolines to synthetically versatile tetrahydroquinoline molecules with I-2 and HBpin is described. In the presence of iodine (20 mol%) as a... 
GALIPEA-OFFICINALIS | HYDROGENATION | SILYLATIVE REDUCTION | PYRIDINES | INHIBITORS | CHEMISTRY, MULTIDISCIPLINARY | INDOLES | N-HETEROARENES | ALKALOIDS | WATER | Chemical reduction | Reagents | Iodine | Organic compounds
Journal Article
Chemical Science, ISSN 2041-6520, 01/2017, Volume 8, Issue 11, pp. 7412 - 7418
The functionalization of heteroarenes has been integral to the structural diversification of medicinally active molecules such as quinolines, pyridines, and... 
Pyridines | Free radicals | Oxidants | Initiators | Oxidizing agents | Catalysis | Ethers | Alkylation | Alcohols | Organic compounds
Journal Article
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