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1. Full Text Intermolecular C–H Silylation of Arenes and Heteroarenes with HSiEt3 under Operationally Diverse Conditions: Neat/Stoichiometric and Acceptor/Acceptorless
by Lee, Kang-sang and Katsoulis, Dimitris and Choi, Jongwook
ACS Catalysis, ISSN 2155-5435, 03/2016, Volume 6, Issue 3, pp. 1493 - 1496
Efficient protocols for Rh-catalyzed intermolecular C–H silylation of unactivated arenes and heteroarenes are disclosed. The silylations are catalyzed by a... 
C-H bond activation | acceptorless C-H silylation | intermolecular C-H silylation | silylation of unactivated arenes and heteroarenes | Rh-catalyzed silylation | C-H silylation | ACTIVATION | CROSS-COUPLING REACTION | SILICON | CHEMISTRY, PHYSICAL | NICKEL-CATALYZED REACTIONS | CLEAVAGE | AROMATIC-COMPOUNDS | FUNCTIONALIZATION | UNACTIVATED C(SP)-H BONDS | ARYLTRIMETHYLSILANES | DEHYDROGENATIVE SILYLATION
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2. Full Text Recent Advances in Transition-Metal-Catalyzed Silylations of Arenes with Hydrosilanes: C–X Bond Cleavage or C–H Bond Activation­ Synchronized with Si–H Bond Activation
by Xu, Zheng and Huang, Wei-Sheng and Zhang, Jin and Xu, Li-Wen
Synthesis, ISSN 0039-7881, 12/2015, Volume 47, Issue 23, pp. 3645 - 3668
Abstract Arylsilanes are valuable organosilicon compounds and attract significant research interest due to their promising applications in organic synthesis.... 
short review | cross-coupling | arylsilanes | homogeneous catalysis | silylation | transition metal | FLUORIDE-MEDIATED CARBOXYLATION | ENANTIOSELECTIVE SYNTHESIS | PALLADIUM-CATALYZED SILYLATION | CHEMISTRY, ORGANIC | SYNTHETIC ROUTE | AROMATIC-COMPOUNDS | DEHYDROGENATIVE SILYLATION | RHODIUM(I)-CATALYZED SILYLATION | ARYL HALIDES | SELECTIVE ARYLATION | TERTIARY SILANES
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3. Full Text Experimental and Computational Exploration of para-Selective Silylation with a Hydrogen-Bonded Template
by Maji, A and Guin, S and Feng, S and Dahiya, A and Singh, VK and Liu, P and Maiti, D
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, ISSN 1433-7851, 11/2017, Volume 56, Issue 47, pp. 14903 - 14907
The regioselective conversion of C-H bonds into C-Si bonds is extremely important owing to the natural abundance and non-toxicity of silicon. Classical... 
regioselectivity | PALLADIUM | ACTIVATION | ARENES | reaction mechanisms | CLEAVAGE | C-H SILYLATION | CATALYZED SILYLATION | CHEMISTRY, MULTIDISCIPLINARY | FUNCTIONALIZATION | hydrogen bonding | CROSS-COUPLING REACTIONS | C-H activation | silylation | UNACTIVATED PRIMARY | ARYL
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4. Full Text Experimental and Computational Studies on Remote γ‑C(sp3)–H Silylation and Germanylation of Aliphatic Carboxamides
by Deb, Arghya and Singh, Sukriti and Seth, Kapileswar and Pimparkar, Sandeep and Bhaskararao, Bangaru and Guin, Srimanta and Sunoj, Raghavan B and Maiti, Debabrata
ACS Catalysis, ISSN 2155-5435, 12/2017, Volume 7, Issue 12, pp. 8171 - 8175
A Pd­(II)-catalyzed protocol for highly regioselective distal γ-C–H silylation and germanylation of aliphatic carboxylic acids is reported. Bidentate... 
germanylation | organopalladium crystal | mechanistic studies | DFT | silylation | γ-C-H activation | DIRECTING GROUP | gamma-C-H activation | CHEMISTRY, PHYSICAL | ALPHA-AMINO-ACIDS | QUATERNARY CARBON CENTERS | C-H BONDS | UNACTIVATED C(SP)-H BONDS | CATALYZED REGIOSELECTIVE SILYLATION | BIS-SILYLATION | organopalladium aystal | INTERMOLECULAR SILYLATION | STEREOSELECTIVE-SYNTHESIS | CARBOXYLIC-ACID DERIVATIVES
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5. Full Text Iridium-Catalyzed, β‑Selective C(sp3)–H Silylation of Aliphatic Amines To Form Silapyrrolidines and 1,2-Amino Alcohols
by Su, Bo and Lee, Taegyo and Hartwig, John F
Journal of the American Chemical Society, ISSN 0002-7863, 12/2018, Volume 140, Issue 51, pp. 18032 - 18038
The functionalization of unactivated C­(sp3)–H bonds of aliphatic amines catalyzed by transition-metal complexes is important because amine-based functionality... 
FUNCTIONALIZATION | ACTIVATION | ENANTIOSELECTIVE SILYLATION | DEHYDROGENATIVE SILYLATION | ARYLATION | NITROGEN | UNACTIVATED C(SP)-H | REGIOSELECTIVE SILYLATION | DIRECTING-GROUP | CHEMISTRY, MULTIDISCIPLINARY | C-H BONDS
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6. Full Text Aryl(triethyl)silanes for Biaryl and Teraryl Synthesis by Copper(II)‐Catalyzed Cross‐Coupling Reaction
by Komiyama, Takeshi and Minami, Yasunori and Hiyama, Tamejiro
Angewandte Chemie International Edition, ISSN 1433-7851, 12/2016, Volume 55, Issue 51, pp. 15787 - 15791
Aryl(triethyl)silanes are found to undergo cross‐coupling with iodoarenes in the presence of catalytic amounts of CuBr2 and Ph‐Davephos, as well as cesium... 
cross-coupling | silanes | copper | arenes | C−H silylation | FLUORINATED BENZOTHIADIAZOLE | GENERAL-SOLUTION | INTRAMOLECULAR ACTIVATION | BUILDING-BLOCKS | CHEMISTRY, MULTIDISCIPLINARY | POLYMER SOLAR-CELLS | DEHYDROGENATIVE SILYLATION | CONJUGATED POLYMERS | C-H silylation | ARYL HALIDES | ORGANIC ELECTRONICS
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7. Full Text Recent Progress in the Cross-Coupling Reaction Using Triorganosilyl-Type Reagents
by Komiyama, Takeshi and Minami, Yasunori and Hiyama, Tamejiro
Synlett, ISSN 0936-5214, 09/2017, Volume 28, Issue 15, pp. 1873 - 1884
The silicon-based cross-coupling reaction has attracted much attention over recent decades because there are many advantages in using organosilicon compounds.... 
nickel | silylation | organosilicon reagents | cross-coupling | copper | palladium | amination | PALLADIUM-CATALYZED SILYLATION | BIARYL SYNTHESIS | CHEMISTRY, ORGANIC | C-H SILYLATION | WHITE ELECTROLUMINESCENCE | LIGHT-EMITTING-DIODES | DIVERSITY-ORIENTED SYNTHESIS | DEHYDROGENATIVE SILYLATION | ARYL HALIDES | AROMATIC HETEROCYCLES | SILOXANE TRANSFER AGENTS
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8. Full Text Recent Progress in the Transition‐Metal‐Catalyzed Activation of Si−Si Bonds To Form C−Si Bonds
by Xiao, Peihong and Gao, Lu and Song, Zhenlei
Chemistry – A European Journal, ISSN 0947-6539, 02/2019, Volume 25, Issue 10, pp. 2407 - 2422
Disilanes possessing a Si−Si bond are unique element–element species. Transition‐metal‐catalyzed activation of the Si−Si bond allows many useful... 
silicon | silylation | Si−Si activation | transition metals | C−Si bond formation | DIRECTING GROUP | H SILYLATION | CHEMISTRY, MULTIDISCIPLINARY | DIRECT INTERMOLECULAR SILYLATION | C-Si bond formation | CROSS-COUPLING REACTIONS | BIS-SILYLATION | AMINO-ACIDS | Si-Si activation | HETEROATOM BONDS | CARBON-CARBON | SILICON-SILICON | STEREOSELECTIVE-SYNTHESIS | Activation | Aromatic compounds | Bonding | Metals
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9. Full Text Friedel–Crafts‐Type Intermolecular C−H Silylation of Electron‐Rich Arenes Initiated by Base‐Metal Salts
by Yin, Qin and Klare, Hendrik F. T and Oestreich, Martin
Angewandte Chemie International Edition, ISSN 1433-7851, 02/2016, Volume 55, Issue 9, pp. 3204 - 3207
An electrophilic aromatic substitution (SEAr) with a catalytically generated silicon electrophile is reported. Essentially any commercially available... 
Lewis acids | hydrosilanes | C−H activation | Si−H activation | electrophilic substitution | C-H activation | Si-H activation | ACTIVATION | COMPLEX | BENZENE | MECHANISM | BOND-CLEAVAGE | CATALYZED SILYLATION | CHEMISTRY, MULTIDISCIPLINARY | INDOLES | FUNCTIONALIZATION | N-SILYLATION | Substitution reactions | Lewis acid | Protons | Salts | Catalysts | Aromatic compounds | Metals | Silicon | Crafts
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10. Full Text Selective C–Si Bond Formation through C–H Functionalization
by Sharma, Ritika and Kumar, Rakesh and Kumar, Inder and Singh, Bikram and Sharma, Upendra
Synthesis, ISSN 0039-7881, 08/2015, Volume 47, Issue 16, pp. 2347 - 2366
Abstract Silylation of hydrocarbons is one of the most important transformations due to the diverse application of organosilanes. Continuous progress is being... 
short review | catalytic | C-H activation | silylation | metal-free | siloles | ORGANIC-SYNTHESIS | C(SP)-H BONDS | ACTIVATION | SILICON-CONTAINING COMPOUNDS | IRIDIUM | HYDROSILANES | CHEMISTRY, ORGANIC | CARBON-HYDROGEN BONDS | CLEAVAGE | CATALYZED REGIOSELECTIVE SILYLATION | DEHYDROGENATIVE SILYLATION
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11. Full Text Broad-spectrum kinetic resolution of alcohols enabled by Cu-H-catalysed dehydrogenative coupling with hydrosilanes
by Dong, Xichang and Weickgenannt, Andreas and Oestreich, Martin
Nature Communications, ISSN 2041-1723, 06/2017, Volume 8, Issue 1, p. 15547
The enantioselective silylation of racemic alcohols, where one enantiomer reacts faster than the other, is an alternative approach to established enzymatic and... 
SILICON-STEREOGENIC SILANES | SECONDARY ALCOHOLS | ENANTIOSELECTIVE SILYLATION | ASYMMETRIC SILYLATION | 1,2-DIOLS | PROTECTION | MULTIDISCIPLINARY SCIENCES | STEREOSELECTIVE SILYLATION | DESYMMETRIZATION
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12. Full Text Palladium-Catalyzed Domino Heck/Silylation Reaction for the Synthesis of (2-Oxoindolin-3-yl)methylsilanes via Trapping of the sigma-Alkylpalladium Intermediates with Disilanes
by Xiao, GH and Chen, L and Zhou, B and Deng, GB and Gong, J and Liang, Y
ADVANCED SYNTHESIS & CATALYSIS, ISSN 1615-4150, 09/2018, Volume 360, Issue 18, pp. 3477 - 3481
A palladium-catalyzed domino Heck/silylation reaction of acrylamides with hexamethyldisilane is presented. This transformation, which involves the formation of... 
Acrylamides | Hexamethyldisilane | DIRECTED ORTHO-METALATION | SILICON | COMPLEXES | CHEMISTRY, ORGANIC | Palladium | OXIDATIVE ADDITION | C-H SILYLATION | silylation | INTERMOLECULAR SILYLATION | ARYL HALIDES | BONDS | Hexamethyldistannane | CHEMISTRY, APPLIED | HECK REACTION | SI-SI
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13. Full Text Pincer Ruthenium Catalyzed Intramolecular Silylation of C(sp2)–H Bonds
by Fang, Huaquan and He, Qiaoxing and Liu, Guixia and Huang, Zheng
Synlett, ISSN 0936-5214, 11/2017, Volume 28, Issue 18, pp. 2468 - 2472
Abstract Reported herein is a highly efficient intramolecular silylation of aromatic C–H bonds catalyzed by a pincer ruthenium complex, giving benzoxasiloles... 
cluster | C-C coupling | ruthenium | pincer ligand | silylation | C-H bond functionalization | TRANSITION-METAL CATALYSIS | ENANTIOSELECTIVE SILYLATION | CHEMISTRY, ORGANIC | CARBON-HYDROGEN BONDS | REGIOSELECTIVE SILYLATION | C-H BONDS | UNACTIVATED C(SP)-H BONDS | CROSS-COUPLING REACTIONS | DEHYDROGENATIVE SILYLATION | ACETAL DIRECTING GROUPS | SILOXANE TRANSFER AGENTS
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14. Full Text Rhodium‐Catalyzed Enantioselective Silylation of Cyclopropyl C−H Bonds
by Lee, Taegyo and Hartwig, John F
Angewandte Chemie International Edition, ISSN 1433-7851, 07/2016, Volume 55, Issue 30, pp. 8723 - 8727
Hydrosilyl ethers, generated in situ by the dehydrogenative silylation of cyclopropylmethanols with diethylsilane, undergo asymmetric, intramolecular... 
cyclopropanes | asymmetric catalysis | C−H activation | silylation | rhodium | ACTIVATION | HYDROSILYLATION | COMPLEXES | ARYLATION | REGIOSELECTIVE SILYLATION | CHEMISTRY, MULTIDISCIPLINARY | FUNCTIONALIZATION | UNACTIVATED C(SP)-H BONDS | C-H activation | DEHYDROGENATIVE SILYLATION | DERIVATIVES | ACCESS | Cyclopropanes - chemistry | Silanes - chemistry | Stereoisomerism | Catalysis | Hydrogen - chemistry | Carbon - chemistry | Rhodium - chemistry | Rhodium | Enantiomers | cyclopropane
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15. Full Text Ruthenium-Catalyzed Site-Selective Intramolecular Silylation of Primary C–H Bonds for Synthesis of Sila-Heterocycles
by Fang, Huaquan and Hou, Wenjun and Liu, Guixia and Huang, Zheng
Journal of the American Chemical Society, ISSN 0002-7863, 08/2017, Volume 139, Issue 33, pp. 11601 - 11609
Incorporating the silicon element into bioactive organic molecules has received increasing attention in medicinal chemistry. Moreover, organosilanes are... 
IRIDIUM PINCER COMPLEXES | UNACTIVATED C(SP)-H BONDS | TRANSITION-METAL CATALYSIS | DEHYDROGENATIVE SILYLATION | ENANTIOSELECTIVE SILYLATION | ORGANIC TRANSFORMATIONS | CARBON/SILICON SWITCH STRATEGY | ACETAL DIRECTING GROUPS | ALKANE DEHYDROGENATION | REGIOSELECTIVE SILYLATION | CHEMISTRY, MULTIDISCIPLINARY
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16. Full Text Iridium-Catalyzed Regioselective C(sp3)–H Silylation of 4‑Alkylpyridines at the Benzylic Position with Hydrosilanes Leading to 4‑(1-Silylalkyl)pyridines
by Fukumoto, Yoshiya and Hirano, Masaya and Chatani, Naoto
ACS Catalysis, ISSN 2155-5435, 05/2017, Volume 7, Issue 5, pp. 3152 - 3156
The regioselective silylation of C­(sp3)–H bonds at the benzylic position in 4-alkylpyridines with hydrosilanes is described. The reaction proceeds in the... 
4-alkylpyridine | hydrosilane | silylation | C-H functionalization | iridium catalyst | PALLADIUM | TRANSITION-METAL-COMPLEXES | ARENES | CHEMISTRY, PHYSICAL | PYRIDINES | AROMATIC-SUBSTITUTION | C-H SILYLATION | DIHYDROGEN COMPLEXES | FUNCTIONALIZATION | DEHYDROGENATIVE SILYLATION | BOND ACTIVATION
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17. Full Text Site-Selective Silylation of Aliphatic C–H Bonds Mediated by [1,5]-Hydrogen Transfer: Synthesis of α‑Sila Benzamides
by Liu, Pei and Tang, Jinghua and Zeng, Xiaoming
Organic Letters, ISSN 1523-7060, 11/2016, Volume 18, Issue 21, pp. 5536 - 5539
The first example of site-selective silylation of C­(sp3)–H bonds mediated by a [1,5]-hydrogen transfer is reported. This reaction occurs selectively at the... 
FUNCTIONALIZATION | NICKEL/MAGNESIUM BIMETALLIC COOPERATION | UNACTIVATED C(SP)-H BONDS | CATALYZED ENANTIOSELECTIVE SILYLATION | DEHYDROGENATIVE SILYLATION | NICKEL | HYDROSILANES | CHEMISTRY, ORGANIC | REGIOSELECTIVE SILYLATION | CLEAVAGE | GRIGNARD-REAGENTS
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18. Full Text Iridium-catalyzed silylation of unactivated C–H bonds
by Hartwig, John F and Romero, Erik A
Tetrahedron, ISSN 0040-4020, 08/2019, Volume 75, Issue 31, pp. 4059 - 4070
The functionalization of primary C–H bonds has been a longstanding challenge in catalysis. Our group has developed a series of silylations of primary C–H bonds... 
Natural product | Oxidation | Iridium | Silylation | C–H bond functionalization | ACTIVATION | DIRECTED HYDROXYLATION | HYDROSILANES | CHEMISTRY, ORGANIC | REGIOSELECTIVE SILYLATION | C-H bond functionalization | FUNCTIONALIZATION | INTERMOLECULAR SILYLATION | DIVERGENT | GERMANYLATION | BORYLATION | Bonds | Catalysis
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19. Full Text B(C6F5)(3)-Catalyzed (Convergent) Disproportionation Reaction of lndoles
by Han, YX and Zhang, ST and He, JH and Zhang, YT
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, ISSN 0002-7863, 05/2017, Volume 139, Issue 21, pp. 7399 - 7407
A metal-free B(C6F5)(3)-catalyzed approach is developed for the disproportionation reaction of a series of indoles with various hydrosilanes, without any... 
ELECTRON | HYDROGENATION | REDUCTION | INDOLINE | ARENES | POLYMERIZATION | HYDROSILATION | AROMATIC-SUBSTITUTION | C-H SILYLATION | CHEMISTRY, MULTIDISCIPLINARY | BOND SILYLATION
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20. Full Text Rhodium-catalyzed intermolecular C-H silylation of arenes with high steric regiocontrol
by Chen, Cheng and Hartwig, John F
Science, ISSN 0036-8075, 2014, Volume 343, Issue 6173, pp. 853 - 857
Regioselective C-H functionalization of arenes has widespread applications in synthetic chemistry. The regioselectivity of these reactions is often controlled... 
ACTIVATION | HETEROARENES | DIRECT ARYLATION | DEHYDROGENATIVE SILYLATION | IRIDIUM COMPLEXES | MULTIDISCIPLINARY SCIENCES | BOND FUNCTIONALIZATION | CLEAVAGE | BORYLATION | INSIGHTS | Chemical reactions | Chemical properties | Research | Rhodium | Chemical research | Catalysts | Molecular biology | Catalysis
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